It sounds like you probably want tall, heavy, and with fluffy feathers (which make it look even bigger than it otherwise would.)Just primarily overall size. Bigger heavier though i do not raise them for meat or eggs. I like big dogs, I have Saints, 8month old pups 107 and 134 pounds. Big cats, Mane Coon, at 25 pounds. Flemish giant rabbits. Toulouse geese. White Holland turkeys just because they are several inches taller than most and two Jersey Giant simply because they have a huge wingspan. Funny i like small cows.
My goal is to breed some of the largest, light buff chickens possible.
To adorn my property.
You will probably just have to try a few different things to see what works. Breeding various directions with what you have is a good starting point.
You might get a few chickens of other breeds that are supposed to be big, raise them up, and see if they are any bigger, or if their chicks are bigger, if you cross them into the ones you have. If you get hens, you can cross them all to your current big rooster and then see which chicks are how close to what you want.
Since you like buff, it would make sense to try other buff breeds first. Buff Cochins are an obvious choice, as are Buff Brahmas. I wonder about Buff Minorcas, too. They are not supposed to be as heavy as the Cochins and Brahmas, but in photos they look rather tall, so they may contribute to a larger overall chicken. For any breed, they might be bigger from one source than another. So you might try getting the same breed from more than one hatchery, or from a hatchery and a private breeder.
If you can't find big enough buffs, yes you certainly could try Jersey Giants. You will get black chicks from the first cross, but breeding those back to buff should give at least a few buffs if you hatch enough chicks, although they may not be very good buffs until a few more generations of selection and breeding.