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Still won't hurt to remove the crust. The protein breaking agent in dish Soap should help loosen it. Like Dawn Dish Soap in warm water.

Try some dish soap in the water to break it up?

@Wyorp Rock @Eggcessive What do you guys think?

If he's scratching it, then it's itchy. Is there any eye at all, or an empty space in the socket?

I think that eye is a goner, & needs to be cleared of dead material, & cleaned out.