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I would go .22 also, except for the firearm discharge laws that apply within city limits. If you hit the coon in the body with a 1000fps pellet gun, it would probably run off and die later of internal bleeding. A .22 would more likely create enough shock to kill it where it stands. If you can...

I assume you are in city limits. Get a 1000fps, scoped pellet gun and shoot the little bastards in the head. Quiet, quick and powerful enough to get the job done. In fact, it is quite enough that you may be able to just shoot them one after another.