Whenever you see those soft-shelled eggs, it means their regular diet or some stressor in their development is causing a lack of calcium...usually it's the latter reason and their regular amount of calcium isn't enough to get them through the crisis~be it molting, poor health, poor nutritive absorption, etc.
Having some OS around is a good idea and feeding their shells back to them is also a good idea. A bag of OS is extremely cheap and lasts a long time, so it's no big thing to have some available to them in hard times. I just plunk the bag in the corner of the coop and rip open the top...they will eat it when they need it, most generally. During molt and into the winter when they are actively regrowing feathers while also using extra nutrition to keep warm, I'll go ahead and add it right in their feed.