What part of the storm was sampled? When the planes do their runs, they report where in the storm the highest wind speeds were recorded. The northeast quadrant is typically the worst. On a northwest course, with the eye passing over the buoy, I would think the nortwest and southeast parts of the storm were the ones that passed over the buoy.
But of course, an airplane can't realistically sample wind speeds at ground level, where even things like waves will create a certain amount of turbulence and drag. The anemometer on bouy 42060 is only 4 meters above the water.